Effect of Carbonization Treatment on Behavior and Mechanism of  Pb2+Adsorption by Recycled Concrete Fines

Abstract

Abstract: With the development of industry, large amounts of lead-containing wastes have been discharged into the environment, causing severe pollution to water bodies. This study used carbonated recycled concrete fines (CRCF) as an adsorbent to conduct adsorption tests on lead contaminated solutions prepared with lead nitrate, and tested and analyzed its phase, microstructure, and stability of CRCF. The results indicated that CRCF possessed outstanding adsorption capacity for Pb²⁺, achieving a removal rate of 93.1% (mass fraction, the same below) after 24 h. The CRCF has high adsorption stability for Pb²⁺, with only negligible amounts of Pb²⁺ leaching after adsorption. In the adsorption reaction, Pb²⁺is electrostatically adsorbed on the surface of CRCF, undergoes ion exchange with CRCF, and forms carbonate precipitation on the surface, ultimately mainly fixed in the form of carbonate in CRCF. CRCF can be used as a low-cost and efficient adsorbent for Pb²⁺, which can be effectively applied to the treatment of lead containing wastewater and achieve waste resource reuse.

Key words: carbonization, recycled concrete fines, adsorption, Pb²⁺, stability

CLC Number:

TU528

WANG Kaiyuan, XIAO Zhenpo, KOU Shicong, WANG Yaocheng, ZHAN Baojian, XING Feng. Effect of Carbonization Treatment on Behavior and Mechanism of Pb²⁺Adsorption by Recycled Concrete Fines[J]. BULLETIN OF THE CHINESE CERAMIC SOCIETY, 2024, 43(4): 1420-1426.

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Effect of Carbonization Treatment on Behavior and Mechanism of Pb²⁺Adsorption by Recycled Concrete Fines

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