Review on CO2 Mineral Carbonation-Cured Cement-Based Materials

Abstract

Abstract: CO₂ mineralization curing is considered an effective approach to mitigate the impact of the construction industry on global climate change by reacting CO₂ with cement-based materials (CBM) (e.g. cement clinker, namely tricalcium silicate, β-dicalcium silicate, tricalcium aluminate and its hydration products, namely calcium hydroxide, amorphous calcium silicate hydrates, hydrated aluminate and sulfate phases) to form calcium carbonate mainly composed of calcite and amorphous silica gel with high degree of polymerization, realizing the storage and utilization of CO₂. Attributed to the good stability, filling effect and nucleation effect of the resultant products, the mechanical properties and durability of CBM are effectively improved while better performance is anticipated in a relatively short time compared with other curing technologies. In this paper, the reaction mechanisms and latest research progress of CO₂ mineral carbonation-cured CBM are reviewed. The effect of influencing factors, such as pre-condition, relative humidity, water binder ratio, CO₂ concentration, curing pressure and temperature on the post-mineralization properties, carbon fixation rate and mineralization degree are evaluated. Finally, based on the current research status and existing problems, suggestions and recommendations for a wider application of CO₂ mineralization technology in the future are also provided.

Key words: carbon dioxide storage and utilization, mineral carbonation curing, cement-based material, reaction mechanism, influencing factor

CLC Number:

X701
TU528

WU Shengkun, HUANG Tianyong, XIE Yan, WANG Zhanpeng, BAO Qi, TIONG Michelle, YE Hang, LIU Qi. Review on CO₂ Mineral Carbonation-Cured Cement-Based Materials[J]. BULLETIN OF THE CHINESE CERAMIC SOCIETY, 2023, 42(6): 1897-1911.

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Review on CO₂ Mineral Carbonation-Cured Cement-Based Materials

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